Sometimes we want to assign or unassign a specific contact to a staff member; there are a couple different ways to do so:
Individual contacts:
Go to the contact profile and change the group in the contact information
List assigned Staff:
Go to the contact group list and choose the contact you want to assign to a staff member:
Click on "Assign Staff" and choose the action you want do, either assign or unassign the contact to a staff member.